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dc.contributor.authorFasshauer, Elke
dc.date.accessioned2017-03-08T14:34:06Z
dc.date.available2017-03-08T14:34:06Z
dc.date.issued2016-04-19
dc.description.abstractInteratomic Coulombic decay (ICD) is an electronic decay process of excited, ionized systems. It has been shown to occur in a multitude of small and large systems. The effects of more than one possible decay partner are discussed in detail illustrated by simulated ICD electron spectra of NeAr clusters and pure Ne clusters. Hereby, the mostly underestimated contribution of decay with non-nearest neighbours is highlighted. In the neon clusters, the lifetime of the bulk atoms is found to be in excellent agreement with experiment (Jahnke et al 2004 Phys. Rev. Lett. 93 173401) while the lifetimes of the surface atoms differ significantly. Hence, the experimental lifetime can not purely be explained by the effect of the number of neighbours. We propose the possibility to investigate the transition from small clusters to the solid state by using the ICD electron spectra to distinguish between icosahedral and cuboctahedral cluster structures.en_US
dc.descriptionPublished version. Source at <a href=http://doi.org/10.1088/1367-2630/18/4/043028>http://doi.org/10.1088/1367-2630/18/4/043028</a>. License <a href=https://creativecommons.org/licenses/by/3.0/>CC BY 3.0</a>.en_US
dc.identifier.citationFasshauer E. Non-nearest neighbour ICD in clusters. New Journal of Physics. 2016;18(4)en_US
dc.identifier.cristinIDFRIDAID 1367010
dc.identifier.doi10.1088/1367-2630/18/4/043028
dc.identifier.issn1367-2630
dc.identifier.urihttps://hdl.handle.net/10037/10482
dc.language.isoengen_US
dc.publisherIOP Publishing Ltden_US
dc.publisherDeutsche Physikalische Gesellschaften_US
dc.relation.journalNew Journal of Physics
dc.relation.projectIDinfo:eu-repo/grantAgreement/RCN/FundingProgram/179568/Norway///en_US
dc.rights.accessRightsopenAccessen_US
dc.subjectVDP::Mathematics and natural science: 400::Physics: 430en_US
dc.subjectinteratomic coulombic decayen_US
dc.subjectneon clustersen_US
dc.subjectNeAr clustersen_US
dc.subjectlifetimesen_US
dc.subjectbulk and surface atomsen_US
dc.subjectdecay widthsen_US
dc.subjecticosahedral versus cuboctahedral structureen_US
dc.titleNon-nearest neighbour ICD in clustersen_US
dc.typeJournal articleen_US
dc.typeTidsskriftartikkelen_US
dc.typePeer revieweden_US


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